Plastidip is probably a fine choice as long as you prep the surface properly (thorough cleaning with alcohol).
Overtime though, the dip will loose its "dipness" and become more and more difficult to remove, particularly with the heat from the headlight so you will want to spray it on extra thick to counteract this.
I would probably just paint it for fear of the dip starting to peel on me or something and having to open the lights back up to fix it.
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